Films
- Greetings - 1968 - Jon Rubin
- Sam's Song - 1969 - Sam
- The Wedding Party - 1969 - Cecil
- Bloody Mama - 1970 - Lloyd Barker
- Hi, Mom! - 1970 - Jon Rubin
- Born to Win - 1971 - Officer Danny
- The Gang That Couldn't Shoot Straight - 1971 - Mario Trantino
- Bang the Drum Slowly - 1973 - Bruce Pearson
- Mean Streets - 1973 - John "Johnny Boy" Civello
- The Godfather Part II - 1974 - Vito Corleone
- Taxi Driver - 1976 - Travis Bickle
- 1900 - 1976 - Alfredo Berlinghieri
- The Last Tycoon - 1976 - Monroe Stahr
- New York, New York - 1977 - Jimmy Doyle
- The Deer Hunter - 1978 - Michael Vronsky
- Raging Bull - 1980 - Jake LaMotta
- True Confessions - 1981 - Monsignor Desmond "Des" Spellacy
- The King of Comedy - 1983 - Rupert Pupkin
- Once Upon a Time in America - 1984 - David "Noodles" Aaronson
- Falling in Love - 1984 - Frank Raftis
- Brazil - 1985 - Archibald "Harry" Tuttle
- The Mission - 1986 - Rodrigo Mendoza
- Angel Heart - 1987 - Louis Cyphre
- The Untouchables - 1987 - Al Capone
- Midnight Run - 1988 - Jack Walsh
- Jacknife - 1989 - Josephe "Jacknife" Megessey
- We're No Angels - 1989 - Ned
- Stanley & Iris - 1990 - Stanley Everett Cox
- Goodfellas - 1990 - James "Jimmy" Conway
- Awakenings - 1990 - Leonard Lowe
- Guilty by Suspicion - 1991 - David Merrill
- Backdraft - 1991 - Donald "Shadow" Rimgale
- Cape Fear - 1991 - Maximilian "Max" Cady
- Night and the City - 1992 - Harry Fabian
- Mistress - 1992 - Evan M. Wirght
- A Bronx Tale - 1993 - Lorenzo Anello
- Mad Dog and Glory - 1993 - Wayne "Mad Dog" Dobie
- This Boy's Life - 1993 - Dwight Hansen
- Mary Shelley's Frankenstein - 1994 - The Creature
- Casino - 1995 - Sam " Ace" Rothstein
- Heat - 1995 - Neil McCauley
- The Fan - 1996 - Gilbert "Gil" Renard
- Sleepers - 1996 - Father Bobby
- Marvin's Room - 1996 - Dr. Wally
- Cop Land - 1997 - Lt. Moe Tilden
- Jackie Brown - 1997 - Louis Gara
- Wag the Dog - 1997 - Conrad Brean
- Great Expectations - 1998 - Arthur Lustig
- Ronin - 1998 - Sam
- Analyze This - 1999 - Paul Vitti
- Flawless - 1999 - Walter Koontz
- The Adventures of Rocky and Bullwinkle - 2000 - Fearless Leader
- Men of Honor - 2000 - Chief Leslie William "Billy" Sunday
- Meet the Parents - 2000 - Jack Tiberius Byrnes
- 15 Minutes - 2001 - Det. Eddie Flemming
- The Score - 2001 - Nick Wells
- Showtime - 2002 - Det. Mitch Preston
- City by the Sea - 2002 - Vincent Anthony LaMarca
- Analyze That - 2002 - Paul Vitti
- Godsend - 2004 - Dr. Richard Wells
- Shark Tale - 2004 - Don Lino (voice)
- Meet the Fockers - 2004 - Jack Tiberius Byrnes
- Hide and Seek - 2005 - David Callaway/Charlie
- Arthur and the Invisibles - 2006 - The King (voice)
- The Good Shepherd - 2006 - General Bill Sullivan
- Stardust - 2007 - Captain Shakespeare
- Righteous Kill - 2008 - Det. Thomas "Turk" Cowan
- What Just Happened - 2008 - Ben
- Everybody's Fine - 2009 - Frank
- Blaze: The Dark Beginning - 2009 - Aldo Gambodi Jr.
- Machete - 2010 - Senator McLaughlin
- Stone - 2010 - Jack Mabry
- Little Fockers - 2010 - Jack Tiberius Byrnes
- Manuale d'amore 3 - 2011 - Adrian
- Killer Elite - 2011 - Hunter
- Limitless - 2011 - Carl Van Loon
- New Year's Eve - 2011 - Stan Harris
- Being Flynn - 2012 - Jonathan Flynn
- Red Lights - 2012 - Simon Silver
- Freelancers - 2012 - Sarcone
- Silver Linings Playbook - 2012 - Pat Solitano, Sr.
- The Big Wedding - 2013 - Don Griffin
- Killing Season - 2013 - Benjamin Ford
- The Family - 2013 - Fred Blake/Giovanni Manzoni
- Last Vegas - 2013 - Paddy
- Grudge Match - 2013 - Billy "The Kid" McGuigan
- Motel - 2013 - Unknown
- Uncharted: Drake's Fortune - 2013 - Victor Sullivan
- The Forgotten Character Forest - 2013 - Fix-It Felix Sr. (voice)
- Blaze 3 - 2013 - Aldo Gambodi Jr.
- Halloween - 2013 - Dr. Samuel Loomis
- Hands of Stone - 2014 - Ray Arcel
- Uncharted 2: Among Thieves - 2014 - Victor Sullivan
- Maiden Voyage - 2014 - Thomas Marshal
- Halloween 2 - 2014 - Dr. Samuel Loomis
- The Knife Of Never Letting Go - 2014 - Peter Stormware
- Jak and Daxter - 2014 - Samos
- The Irishman - 2015 - Frank Sheeran
- Halloween 4 3D - 2015 - Earl
- Jak 2 - 2015 - Samos
- Jak 3 - 2016 - Samos
- Jak X - 2017 - Samos
- Jak 4: The Darkness Within - 2019 - Samos
- Jak 5: The Full Moon - 2020 - Samos
- The Prince Of The Dinosaurs - Spirit Tree
- Jak 6 - 2021 - Samos
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